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Chern, G. W., & Mellado, P. (2016). Magnetic monopole polarons in artificial spin ices. Epl, 114(3), 6 pp.
Abstract: Emergent quasiparticles that arise from the fractionalization of the microscopic degrees of freedom have been one of the central themes in modern condensed-matter physics. The notion of magnetic monopoles, freely moving quasiparticles fragmented from local dipole excitations, has enjoyed much success in understanding the thermodynamic, static, and transport properties of the so-called spin-ice materials. The artificial version of spin ice, where a lattice of nanoscale magnetic dipoles is sculpted out of a ferromagnetic film, provides a unique opportunity to study these unusual quasiparticles in a material-by-design approach. Here we show that the elementary excitations in the ice phase of a nano-magnetic array arranged in the pentagonal lattice are composite objects comprised of the emergent monopole and a surrounding cloud of opposite uncompensated magnetic charges. Copyright (C) EPLA, 2016
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Cisternas, J., Mellado, P., Urbina, F., Portilla, C., Carrasco, M., & Concha, A. (2021). Stable and unstable trajectories in a dipolar chain. Phys. Rev. B, 103(13), 134443.
Abstract: In classical mechanics, solutions can be classified according to their stability. Each of them is part of the possible trajectories of the system. However, the signatures of unstable solutions are hard to observe in an experiment, and most of the times if the experimental realization is adiabatic, they are considered just a nuisance. Here we use a small number of XY magnetic dipoles subject to an external magnetic field for studying the origin of their collective magnetic response. Using bifurcation theory we have found all the possible solutions being stable or unstable, and explored how those solutions are naturally connected by points where the symmetries of the system are lost or restored. Unstable solutions that reveal the symmetries of the system are found to be the culprit that shape hysteresis loops in this system. The complexity of the solutions for the nonlinear dynamics is analyzed using the concept of boundary basin entropy, finding that the damping timescale is critical for the emergence of fractal structures in the basins of attraction. Furthermore, we numerically found domain wall solutions that are the smallest possible realizations of transverse walls and vortex walls in magnetism. We experimentally confirmed their existence and stability showing that our system is a suitable platform to study domain wall dynamics at the macroscale.
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Concha, A., Aguayo, D., & Mellado, P. (2018). Designing Hysteresis with Dipolar Chains. Phys. Rev. Lett., 120(15), 5 pp.
Abstract: Materials that have hysteretic response to an external field are essential in modern information storage and processing technologies. A myriad of magnetization curves of several natural and artificial materials have previously been measured and each has found a particular mechanism that accounts for it. However, a phenomenological model that captures all the hysteresis loops and at the same time provides a simple way to design the magnetic response of a material while remaining minimal is missing. Here, we propose and experimentally demonstrate an elementary method to engineer hysteresis loops in metamaterials built out of dipolar chains. We show that by tuning the interactions of the system and its geometry we can shape the hysteresis loop which allows for the design of the softness of a magnetic material at will. Additionally, this mechanism allows for the control of the number of loops aimed to realize multiple-valued logic technologies. Our findings pave the way for the rational design of hysteretical responses in a variety of physical systems such as dipolar cold atoms, ferroelectrics, or artificial magnetic lattices, among others.
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Concha, A., Mellado, P., Morera-Brenes, B., Costa, C. S., Mahadevan, L., & Monge-Najera, J. (2015). Oscillation of the velvet worm slime jet by passive hydrodynamic instability. Nat. Commun., 6, 6 pp.
Abstract: The rapid squirt of a proteinaceous slime jet endows velvet worms (Onychophora) with a unique mechanism for defence from predators and for capturing prey by entangling them in a disordered web that immobilizes their target. However, to date, neither qualitative nor quantitative descriptions have been provided for this unique adaptation. Here we investigate the fast oscillatory motion of the oral papillae and the exiting liquid jet that oscillates with frequencies f similar to 30-60 Hz. Using anatomical images, high-speed videography, theoretical analysis and a physical simulacrum, we show that this fast oscillatory motion is the result of an elastohydrodynamic instability driven by the interplay between the elasticity of oral papillae and the fast unsteady flow during squirting. Our results demonstrate how passive strategies can be cleverly harnessed by organisms, while suggesting future oscillating microfluidic devices, as well as novel ways for micro and nanofibre production using bioinspired strategies.
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Farhan, A., Petersen, C. F., Dhuey, S., Anghinolfi, L., Qin, Q. H., Saccone, M., et al. (2017). Nanoscale control of competing interactions and geometrical frustration in a dipolar trident lattice. Nat. Commun., 8, 7 pp.
Abstract: Geometrical frustration occurs when entities in a system, subject to given lattice constraints, are hindered to simultaneously minimize their local interactions. In magnetism, systems incorporating geometrical frustration are fascinating, as their behavior is not only hard to predict, but also leads to the emergence of exotic states of matter. Here, we provide a first look into an artificial frustrated system, the dipolar trident lattice, where the balance of competing interactions between nearest-neighbor magnetic moments can be directly controlled, thus allowing versatile tuning of geometrical frustration and manipulation of ground state configurations. Our findings not only provide the basis for future studies on the low-temperature physics of the dipolar trident lattice, but also demonstrate how this frustration-by-design concept can deliver magnetically frustrated metamaterials.
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Farhan, A., Scholl, A., Petersen, C. F., Anghinolfi, L., Wuth, C., Dhuey, S., et al. (2016). Thermodynamics of emergent magnetic charge screening in artificial spin ice. Nat. Commun., 7, 6 pp.
Abstract: Electric charge screening is a fundamental principle governing the behaviour in a variety of systems in nature. Through reconfiguration of the local environment, the Coulomb attraction between electric charges is decreased, leading, for example, to the creation of polaron states in solids or hydration shells around proteins in water. Here, we directly visualize the real-time creation and decay of screened magnetic charge configurations in a two-dimensional artificial spin ice system, the dipolar dice lattice. By comparing the temperature dependent occurrence of screened and unscreened emergent magnetic charge defects, we determine that screened magnetic charges are indeed a result of local energy reduction and appear as a transient minimum energy state before the system relaxes towards the predicted ground state. These results highlight the important role of emergent magnetic charges in artificial spin ice, giving rise to screened charge excitations and the emergence of exotic low-temperature configurations.
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Mellado, P. (2020). Timescales in the thermal dynamics of magnetic dipolar clusters. Phys. Rev. B, 102(21), 214442.
Abstract: The collective behavior of thermally active structures offers clues on the emergent degrees of freedom and the physical mechanisms that determine the low-energy state of a variety of systems. Here, the thermally active dynamics of magnetic dipoles at square plaquettes is modeled in terms of Brownian oscillators in contact with a heat bath. Solution of the Langevin equation for a set of interacting x-y dipoles allows the identification of the timescales and correlation length that reveal how interactions, temperature, damping, and inertia may determine the frequency modes of edge and bulk magnetic mesospins in artificial dipolar systems.
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Mellado, P. (2022). Intrinsic topological magnons in arrays of magnetic dipoles. Sci. Rep., 12(1), 1420.
Abstract: We study a simple magnetic system composed of periodically modulated magnetic dipoles with an easy axis. Upon adjusting the geometric modulation amplitude alone, chains and two-dimensional stacked chains exhibit a rich magnon spectrum where frequency gaps and magnon speeds are easily manipulable. The blend of anisotropy due to dipolar interactions between magnets and geometrical modulation induces a magnetic phase with fractional Zak number in infinite chains and end states in open one-dimensional systems. In two dimensions it gives rise to topological modes at the edges of stripes. Tuning the amplitude in two-dimensional lattices causes a band touching, which triggers the exchange of the Chern numbers of the volume bands and switches the sign of the thermal conductivity.
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Mellado, P. (2022). Topological edge states in dipolar zig-zag stripes. J. Phys. Materials, 5(3), 034007.
Abstract: We study the magnon spectrum of stacked zig-zag chains of point magnetic dipoles with an easy axis. The anisotropy due to the dipolar interactions and the two-point basis of the zig-zag chain unit cell combine to give rise to topologically non-trivial magnon bands in 2D zig-zag lattices. Adjusting the distance between the two sublattice sites in the unit cell causes a band touching, which triggers the exchange of the Chern numbers of volume bands switching the sign of the thermal conductivity and the sense of motion of edges modes in zig-zag stripes. We show that these topological features survive when the range of the dipolar interactions is truncated up to the second nearest neighbors.
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Mellado, P., & Tapia, I. (2023). Magnetic solitons due to interfacial chiral interactions. J. Phys. Condens. Matter, 35(16), 164002.
Abstract: We study solitons in a zig-zag lattice of magnetic dipoles. The lattice comprises two sublattices of parallel chains with magnetic dipoles at their vertices. Due to orthogonal easy planes of rotation for dipoles belonging to different sublattices, the total dipolar energy of this system is separable into a sum of symmetric and chiral long-ranged interactions between the magnets where the last takes the form of Dzyaloshinskii-Moriya (DM) coupling. For a specific range of values of the offset between sublattices, the dipoles realize an equilibrium magnetic state in the lattice plane, consisting of one chain settled in an antiferromagnetic (AF) parallel configuration and the other in a collinear ferromagnetic fashion. If the offset grows beyond this value, the internal DM field stabilizes two Bloch domain walls at the edges of the AF chain. The dynamics of these solitons is studied by deriving the long-wavelength lagrangian density for the easy axis antiferromagnet. We find that the chiral couplings between sublattices give rise to an effective magnetic field that stabilizes the solitons in the antiferromagnet. When the chains displace respect to each other, an emergent Lorentz force accelerates the domain walls along the lattice.
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Mellado, P., Concha, A., Hofhuis, K., & Tapia, I. (2023). Intrinsic chiral field as vector potential of the magnetic current in the zig-zag lattice of magnetic dipoles. Sci. Rep., 13(1), 1245.
Abstract: Chiral magnetic insulators manifest novel phases of matter where the sense of rotation of the magnetization is associated with exotic transport phenomena. Effective control of such phases and their dynamical evolution points to the search and study of chiral fields like the Dzyaloshinskii-Moriya interaction. Here we combine experiments, numerics, and theory to study a zig-zag dipolar lattice as a model of an interface between magnetic in-plane layers with a perpendicular magnetization. The zig-zag lattice comprises two parallel sublattices of dipoles with perpendicular easy plane of rotation. The dipolar energy of the system is exactly separable into a sum of symmetric and antisymmetric long-range exchange interactions between dipoles, where the antisymmetric coupling generates a nonlocal Dzyaloshinskii-Moriya field which stabilizes winding textures with the form of chiral solitons. The Dzyaloshinskii-Moriya interaction acts as a vector potential or gauge field of the magnetic current and gives rise to emergent magnetic and electric fields that allow the manifestation of the magnetoelectric effect in the system.
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Mellado, P., Concha, A., & Rica, S. (2020). Magnetoelectric Effect in Dipolar Clusters. Phys. Rev. Lett., 125(23), 237602.
Abstract: We combine the anisotropy of magnetic interactions and the point symmetry of finite solids in the study of dipolar clusters as new basic units for multiferroics metamaterials. The Hamiltonian of magnetic dipoles with an easy axis at the vertices of polygons and polyhedra, maps exactly into a Hamiltonian with symmetric and antisymmetric exchange couplings. The last one gives rise to a Dzyaloshinskii-Moriya contribution responsible for the magnetic modes of the systems and their symmetry groups, which coincide with those of a particle in a crystal field with spin-orbit interaction. We find that the clusters carry spin current and that they manifest the magnetoelectric effect. We expect our results to pave the way for the rational design of magnetoelectric devices at room temperature
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Mellado, P., Petrova, O., & Tchernyshyov, O. (2015). Projective symmetry of partons in the Kitaev honeycomb model. Phys. Rev. B, 91(4), 4 pp.
Abstract: Low-energy states of quantum spin liquids are thought to involve partons living in a gauge-field background. We study the spectrum of Majorana fermions of the Kitaev honeycomb model on spherical clusters. The gauge field endows the partons with half-integer orbital angular momenta. As a consequence, the multiplicities do not reflect the point-group symmetries of the cluster, but rather its projective symmetries, operations combining physical and gauge transformations. The projective symmetry group of the ground state is the double cover of the point group.
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Owerre, S. A., Mellado, P., & Baskaran, G. (2019). Photoinduced Floquet topological magnons in Kitaev magnets. Epl, 126(2), 7 pp.
Abstract: We study periodically driven pure Kitaev model and ferromagnetic phase of the Kitaev-Heisenberg model on the honeycomb lattice by off-resonant linearly and circularly polarized lights at zero magnetic field. Using a combination of linear spin wave and Floquet theories, we show that the effective time-independent Hamiltonians in the off-resonant regime map onto the corresponding anisotropic static spin model, plus a tunable photoinduced magnetic field along the [111] direction, which precipitates Floquet topological magnons and chiral magnon edge modes. They are tunable by the light amplitude and polarization. Similarly, we show that the thermal Hall effect induced by the Berry curvature of the Floquet topological magnons can also be tuned by the laser field. Our results pave the way for ultrafast manipulation of topological magnons in irradiated Kitaev magnets, and could play a pivotal role in the investigation of ultrafast magnon spin current generation in Kitaev materials. Copyright (C) EPLA, 2019
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Petrova, O., Mellado, P., & Tchernyshyov, O. (2013). Unpaired Majorana modes in the gapped phase of Kitaev's honeycomb model. Phys. Rev. B, 88(14), 4 pp.
Abstract: We study the gapped phase of Kitaev's honeycomb model (a Z(2) spin liquid) in the presence of lattice defects. We find that some dislocations and bond defects carry unpaired Majorana fermions. Physical excitations associated with these defects are (complex) fermion modes made out of two (real) Majorana fermions connected by a Z(2) gauge string. The quantum state of these modes is robust against local noise and can be changed by winding a Z(2) vortex around a dislocation. The exact solution respects gauge invariance and reveals a crucial role of the gauge field in the physics of Majorana modes.
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Petrova, O., Mellado, P., & Tchernyshyov, O. (2014). Unpaired Majorana modes on dislocations and string defects in Kitaev's honeycomb model. Phys. Rev. B, 90(13), 14 pp.
Abstract: We study the gapped phase of Kitaev's honeycomb model (a Z(2) spin liquid) on a lattice with topological defects. We find that some dislocations and string defects carry unpaired Majorana fermions. Physical excitations associated with these defects are (complex) fermion modes made out of two (real) Majorana fermions connected by a Z(2) gauge string. The quantum state of these modes is robust against local noise and can be changed by winding a Z(2) vortex around one of the dislocations. The exact solution respects gauge invariance and reveals a crucial role of the gauge field in the physics of Majorana modes. To facilitate these theoretical developments, we recast the degenerate perturbation theory for spins in the language of Majorana fermions.
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Rademaker, L., & Mellado, P. (2018). Charge-transfer insulation in twisted bilayer graphene. Phys. Rev. B, 98(23), 7 pp.
Abstract: We studied the real-space structure of states in twisted bilayer graphene at the magic angle theta = 1.08 degrees. The flat bands close to charge neutrality are composed of a mix of “ring” and “center” orbitals around the AA stacking region. An effective model with localized orbitals is constructed which necessarily includes more than just the four flat bands. Long-range Coulomb interaction causes a charge transfer at half filling of the flat bands from the center to the ring orbitals. Consequently, the Mott phase is a featureless spin-singlet paramagnet. We estimate the effective Heisenberg coupling that favors the singlet coupling to be J = 3.3 K, consistent with experimental values. The superconducting state depends on the nature of the dopants: hole-doping yields (p + ip)-wave, whereas electron-doping yields (d + id)-wave pairing symmetry.
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Rademaker, L., Abanin, D. A., & Mellado, P. (2019). Charge smoothening and band flattening due to Hartree corrections in twisted bilayer graphene. Phys. Rev. B, 100(20), 6 pp.
Abstract: Doping twisted bilayer graphene away from charge neutrality leads to an enormous buildup of charge inhomogeneities within each moire unit cell. Here, we show, using unbiased real-space self-consistent Hartree calculations on a relaxed lattice, that Coulomb interactions smoothen this charge imbalance by changing the occupation of earlier identified “ring” orbitals in the AB/BA region and “center” orbitals at the AA region. For hole doping, this implies an increase of the energy of the states at the Gamma point, leading to a further flattening of the flat bands and a pinning of the Van Hove singularity at the Fermi level. The charge smoothening will affect the subtle competition between different possible correlated phases.
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